Catalytic and capacity properties of nanocomposites based on cobalt oxide and nitrogen-doped carbon nanofibers

doi:10.1016/S1872-2067(14)60099-1

催化学报 ›› 2014, Vol. 35 ›› Issue (6): 960-969.DOI: 10.1016/S1872-2067(14)60099-1

Catalytic and capacity properties of nanocomposites based on cobalt oxide and nitrogen-doped carbon nanofibers

Olga Yu. Podyacheva^a, Andrei I. Stadnichenko^a,b, Svetlana A. Yashnik^a, Olga A. Stonkus^a,b, Elena M. Slavinskaya^a, Andrei I. Boronin^a,b, Andrei V. Puzynin^c, Zinfer R. Ismagilov^a,c

a Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, Novosibirsk 630090, Russia;
b Novosibirsk State University, Ul. Pirogova 2, Novosibirsk, 630090, Russia;
c Institute of Coal Chemistry and Material Science, Pr. Sovetskiy 18, Kemerovo 650000, Russia

收稿日期:2014-03-27 修回日期:2014-04-09 出版日期:2014-05-30 发布日期:2014-06-03
通讯作者: Olga Yu. Podyacheva
基金资助:
This work was supported by RFBR Grant 12-03-01091-a, Presidium RAS (Project 24.51), Presidium SB RAS (Project 36, Project 75).

Catalytic and capacity properties of nanocomposites based on cobalt oxide and nitrogen-doped carbon nanofibers

Olga Yu. Podyacheva^a, Andrei I. Stadnichenko^a,b, Svetlana A. Yashnik^a, Olga A. Stonkus^a,b, Elena M. Slavinskaya^a, Andrei I. Boronin^a,b, Andrei V. Puzynin^c, Zinfer R. Ismagilov^a,c

a Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, Novosibirsk 630090, Russia;
b Novosibirsk State University, Ul. Pirogova 2, Novosibirsk, 630090, Russia;
c Institute of Coal Chemistry and Material Science, Pr. Sovetskiy 18, Kemerovo 650000, Russia

Received:2014-03-27 Revised:2014-04-09 Online:2014-05-30 Published:2014-06-03
Supported by:
This work was supported by RFBR Grant 12-03-01091-a, Presidium RAS (Project 24.51), Presidium SB RAS (Project 36, Project 75).

摘要/Abstract

摘要：

The nanocomposites based on cobalt oxide and nitrogen-doped carbon nanofibers (N-CNFs) with cobalt oxide contents of 10-90 wt% were examined as catalysts in the CO oxidation and supercapacity electrodes. Depending on Co₃O₄ content, such nanocomposites have different morphologies of cobalt oxide nanoparticles, distributions over the bulk, and ratios of Co³⁺/Co²⁺ cations. The 90%Co₃O₄-N-CNFs nanocomposite showed the best activity because of the increased concentration of defects in N-CNFs. The capacitance of electrodes containing 10%Co₃O₄-N-CNFs was 95 F/g, which is 1.7 times higher than electrodes made from N-CNFs.

关键词: Cobalt oxide, Nitrogen-doped carbon nanofibers, Nanocomposite, CO oxidation, Capacity

Abstract:

Key words: Cobalt oxide, Nitrogen-doped carbon nanofibers, Nanocomposite, CO oxidation, Capacity

Olga Yu. Podyacheva, Andrei I. Stadnichenko, Svetlana A. Yashnik, Olga A. Stonkus, Elena M. Slavinskaya, Andrei I. Boronin, Andrei V. Puzynin, Zinfer R. Ismagilov. Catalytic and capacity properties of nanocomposites based on cobalt oxide and nitrogen-doped carbon nanofibers[J]. 催化学报, 2014, 35(6): 960-969.

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Catalytic and capacity properties of nanocomposites based on cobalt oxide and nitrogen-doped carbon nanofibers

Catalytic and capacity properties of nanocomposites based on cobalt oxide and nitrogen-doped carbon nanofibers

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