Fe-TiO2 and Fe2O3 quantum dots co-loaded on MCM-41 for removing aqueous rose bengal by combined adsorption/photocatalysis

doi:10.1016/S1872-2067(17)62976-0

Abstract

Abstract:

Adsorption and photodegradation are promising approaches for removing organic pollutions. In this study, we combined these two processes by co-loading Fe-TiO₂ and Fe₂O₃ quantum dots (QDs) on porous MCM-41, using a simple hydrolysis method. X-ray diffraction, high-resolution transmission electron microscopy, and X-ray photoelectron spectroscopy results indicated that Fe-TiO₂ QDs are formed at low Fe precursor concentrations, while additional Fe₂O₃ QDs are formed at higher Fe precursor concentrations. The Fe₂O₃ and Fe-TiO₂ QDs impart high adsorption capacity and high photoactivity to the porous MCM-41, respectively. Thus, their combination results in a synergic effect of the adsorption and photodegradation. The highest-performing sample exhibits excellent performance in removing rose bengal from aqueous solution.

Key words: Quantum dot, Titania, Ferric oxide, Photocatalysis, Adsorption

Guoqiang Shen, Lun Pan, Zhe Lü, Chongqing Wang, Fazal-e-Aleem, Xiangwen Zhang, Ji-Jun Zou. Fe-TiO₂ and Fe₂O₃ quantum dots co-loaded on MCM-41 for removing aqueous rose bengal by combined adsorption/photocatalysis[J]. Chinese Journal of Catalysis, 2018, 39(5): 920-928.

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Fe-TiO₂ and Fe₂O₃ quantum dots co-loaded on MCM-41 for removing aqueous rose bengal by combined adsorption/photocatalysis

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