Decorating Ag/AgCl on UiO-66-NH2: Synergy between Ag plasmons and heterostructure for the realization of efficient visible light photocatalysis

doi:10.1016/S1872-2067(19)63377-2

Abstract

Abstract: UiO-66-NH₂, as typical visible light responsive Zr-based metal-organic frameworks (MOFs), has attracted great interest in recent years. However, rapid combination of the photoinduced carriers limits its further application. Here, we designed a facile precipitation-photoreduction method to post-synthetically decorate Ag/AgCl on the surface of UiO-66-NH₂ and form a heterostructure. Metallic Ag can not only transmit electrons between UiO-66-NH₂ and AgCl but also absorb visible light, because of the surface plasmon resonance (SPR) effect. The rhodamine B photodegradation rate of UiO-66-NH₂/Ag/AgCl (16.2 wt.% Ag) is about 10 and 4 times those of UiO-66-NH₂ and Ag/AgCl, respectively. The SPR effect of Ag NPs and the formation of a heterostructure synergistically increase the absorbability of visible light, accelerate the separation of photoinduced charges, and promote the formation of superoxide radicals. We expect that our work could provide a new viewpoint for constructing efficient MOF-based photocatalytic systems.

Key words: UiO-66-NH₂, Ag/AgCl, Heterostructure, Visible light photocatalysis, Superoxide radical

Wanyue Zhao, Tong Ding, Yating Wang, Moqing Wu, Wenfeng Jin, Ye Tian, Xingang Li. Decorating Ag/AgCl on UiO-66-NH₂: Synergy between Ag plasmons and heterostructure for the realization of efficient visible light photocatalysis[J]. Chinese Journal of Catalysis, 2019, 40(8): 1187-1197.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(19)63377-2

https://www.cjcatal.com/EN/Y2019/V40/I8/1187

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Decorating Ag/AgCl on UiO-66-NH₂: Synergy between Ag plasmons and heterostructure for the realization of efficient visible light photocatalysis

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