Tunable localized surface plasmon resonances in MoO3-x-TiO2 nanocomposites with enhanced catalytic activity for CO2 photoreduction under visible light

doi:10.1016/S1872-2067(20)63566-5

Abstract

Abstract: The photocatalytic reduction of CO₂ with H₂O to fuels and chemicals using solar energy is one of the most attractive but highly difficult routes. Thus far, only a very limited number of photocatalysts has been reported to be capable of catalyzing the photocatalytic reduction of CO₂ under visible light. The utilization of the localized surface plasmon resonance (LSPR) phenomenon is an attractive strategy for developing visible-light photocatalysts. Herein, we have succeeded in synthesizing plasmonic MoO_3-x-TiO₂ nanocomposites with tunable LSPR by a simple solvothermal method. The well-structured nanocomposite containing two-dimensional (2D) molybdenum oxide (MoO_3-x) nanosheets and one-dimensional (1D) titanium oxide nanotubes (TiO₂-NT) showed LSPR absorption band in the visible-light region, and the incorporation of TiO₂-NT significantly enhanced the LSPR absorption band. The MoO_3-x-TiO₂-NT nanocomposite is promising for application in the photocatalytic reduction of CO₂ with H₂O under visible light irradiation.

Key words: Photocatalysis, Carbon dioxide, Visible light, Localized surface plasmon resonance, MoO_3-x-TiO₂ nanocomposite

Shunji Xie, Haikun Zhang, Guodong Liu, Xuejiao Wu, Jinchi Lin, Qinghong Zhang, Ye Wang. Tunable localized surface plasmon resonances in MoO_3-x-TiO₂ nanocomposites with enhanced catalytic activity for CO₂ photoreduction under visible light[J]. Chinese Journal of Catalysis, 2020, 41(7): 1125-1131.

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Tunable localized surface plasmon resonances in MoO_3-x-TiO₂ nanocomposites with enhanced catalytic activity for CO₂ photoreduction under visible light

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