Interfacial Zn-N bond bridges direct S-scheme charge transfer

doi:10.1016/S1872-2067(25)64809-1

Chinese Journal of Catalysis ›› 2025, Vol. 78: 4-6.DOI: 10.1016/S1872-2067(25)64809-1

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Interfacial Zn-N bond bridges direct S-scheme charge transfer

Feiyan Fu^a^,^*(), Yunfeng Li^b^,^*()

Received:2025-07-16 Accepted:2025-07-21 Online:2025-11-18 Published:2025-10-14
About author:Feiyan Fu, State Key Laboratory of Chemistry for NBC Hazards Protection, Beijing 102205, China, E-mail: fufeiyan1@126.com (F. Fu)
Yunfeng Li, College of Environmental and Chemical Engineering, Key Laboratory of Functional Textile Material and Product of the Ministry of Education, Xi’an Polytechnic University, Xi’an 710048, Shannxi, China, E-mail: liyf377@nenu.edu.cn (Y. Li)
Supported by:
National Natural Science Foundation of China(22578345);National Natural Science Foundation of China(22008185);National Natural Science Foundation of China(21872023);Shaanxi Provincial Key Research and Development Program(2022GY-166);Shaanxi Provincial Key Research and Development Program(2024SF-YBXM-593);Shaanxi Provincial Department of Education Youth Innovation Team Research Plan Project(24JP072);Scientific Research Program Funded by Shaanxi Provincial Education Department(23JC033);Xi’an Science and Technology Planning Project(24GXFW0021)

Abstract

Feiyan Fu, Yunfeng Li. Interfacial Zn-N bond bridges direct S-scheme charge transfer[J]. Chinese Journal of Catalysis, 2025, 78: 4-6.

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Fig. 2. (a) XANES spectra for ZnO, ZCOF20, and Zn foil. (b) FT-EXAFS fitting curve for ZnO and ZCOF20 at the Zn K-edge using the structural model of Zn-O4 and Zn-O3N. In-situ irradiated XPS spectra of Zn 2p (c) and N 1s (d) for ZCOF20 as compared with those for ZCOF20, ZnO, and COF in the dark. (e) The distribution pattern of frontier molecular orbitals of COF. (f) Calculated partial density of states of ZnO. (g) Schematic of the interfacial electron transfer and the IEF formation upon hybridization. Reproduced with permission from Ref. [8]. Copyright 2025, Wiley.

Interfacial Zn-N bond bridges direct S-scheme charge transfer

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