Inhibiting Pd nanoparticle aggregation and improving catalytic performance using one-dimensional CeO2 nanotubes as support

doi:10.1016/S1872-2067(12)60536-1

Abstract

Abstract:

One-dimensional (1D) CeO₂ nanotubes can be used as a support to inhibit Pd nanoparticle aggregation during the high temperature calcination process in air. This is in opposition to the significant aggregation of Pd particles that is observed for the preparation of supported Pd metal catalysts using non-1D commercial CeO₂ as support. The as-prepared Pd/CeO₂ nanotube catalyst exhibits much higher catalytic performance than Pd/commercial CeO₂ toward the aerobic selective oxidation of benzyl alcohol to benzaldehyde. This work suggests that 1D metal oxide materials can be used as a promising class of supports to inhibit noble metal nanoparticle aggregation, thereby improving catalytic performance toward target reactions.

Key words: Ceria, Nanotube, Palladium, Nanoparticle, Support effect, Selective oxidation

TANG Zirong, YIN Xia, ZHANG Yanhui, ZHANG Nan, XU Yijun. Inhibiting Pd nanoparticle aggregation and improving catalytic performance using one-dimensional CeO₂ nanotubes as support[J]. Chinese Journal of Catalysis, 2013, 34(6): 1123-1127.

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Inhibiting Pd nanoparticle aggregation and improving catalytic performance using one-dimensional CeO₂ nanotubes as support

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