Selective suppression of toluene formation in solvent-free benzyl alcohol oxidation using supported Pd-Ni bimetallic nanoparticles

doi:10.1016/S1872-2067(17)62904-8

Abstract

Abstract:

The solvent-free oxidation of benzyl alcohol was studied using supported Pd-Ni bimetallic nanopar-ticles. Compared with monometallic Pd, the addition of Ni to Pd was found to be effective in sup-pressing the nondesired product toluene, thereby enhancing the selectivity towards benzaldehyde. This result was attributed to a dual effect of Ni addition:the weakening of dissociative adsorption of benzyl alcohol and the promotion of oxygen species involved in the oxidation pathway.

Key words: Palladium-nickel, Bimetallic nanoparticle, Benzyl alcohol, Toluene, Solvent-free, Oxidation

Jianwei Che, Mengjia Hao, Wuzhong Yi, Hisayoshi Kobayashi, Yuheng Zhou, Liping Xiao, Jie Fan. Selective suppression of toluene formation in solvent-free benzyl alcohol oxidation using supported Pd-Ni bimetallic nanoparticles[J]. Chinese Journal of Catalysis, 2017, 38(11): 1870-1879.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(17)62904-8

https://www.cjcatal.com/EN/Y2017/V38/I11/1870

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