Ordered mesoporous carbon-based titania as a reusable adsorbent-catalyst for removing phenol from water

doi:10.1016/S1872-2067(12)60567-1

Abstract

Abstract:

The high efficiency of ordered mesoporous carbon-based anatase for the visible light-driven photo-degradation of phenol in water is reported. Adsorption-photocatalysis cycles were used to treat polluted water. Contaminated water containing 200 mg/L phenol can be completely mineralized within 10 cycles, in which each cycle consisted of adsorption for 8 h and visible light-driven illumination for 8 h. The roles of non-metal doping in the anatase lattice, aggregation-free confinement of anatase nanoparticles by the carbon pore wall, and adsorption of phenol in the mesopores on the catalytic performance are discussed. The present work provides an effective combination of physical and chemical treatments to remove relatively high concentrations of non-biodegradable organic substances using a mesoporous photocatalyst.

Key words: Phenol, Visible light, Titania, Carbon-doping, Mesoporous photocatalyst

WEI Wei, YU Chao, ZHAO Qingfei, QIAN Xufang, WAN Ying. Ordered mesoporous carbon-based titania as a reusable adsorbent-catalyst for removing phenol from water[J]. Chinese Journal of Catalysis, 2013, 34(6): 1066-1075.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(12)60567-1

https://www.cjcatal.com/EN/Y2013/V34/I6/1066

References

[1] Leong Y K, Sganzerla M, Berndt C C, Campbell G R. Ind Eng Chem Res, 2008, 47: 1380

[2] Moussavi G, Mahmoudi M, Barikbin B. Water Res, 2009, 43: 1295

[3] Lin S H, Juang R S. J Environ Manage, 2009, 90: 1336

[4] Zeng J, Liu S L, Cai J, Zhang L N. J Phys Chem C, 2010, 114: 7806

[5] Su R, Tiruvalam R, He Q, Dimitratos N, Kesavan L, Hammond C, Lopez-Sanchez J A, Bechstein R, Kiely C J, Hutchings G J, Besenbacher F. ACS Nano, 2012, 6: 6284

[6] Kisch H, Zang L, Lange C, Maier W F, Antonius C, Meissner D. Angew Chem, Int Ed, 1998, 37: 3034

[7] Macyk W, Kisch H. Chem-Eur J, 2001, 7: 1862

[8] Park J H, Kim S, Bard A J. Nano Lett, 2006, 6: 24

[9] Sakthivel S, Kisch H. Angew Chem, Int Ed, 2003, 42: 4908

[10] Liu S W, Yu J G, Jaroniec M. J Am Chem Soc, 2010, 132: 11914

[11] Garcia-Amoros J, Finkelmann H, Velasco D. J Mater Chem, 2011, 21: 1094

[12] Dong F, Wang H Q, Wu Z B. J Phys Chem C, 2009, 113: 16717

[13] McEvoy J G, Cui W Q, Zhang Z S. Catal Today, 2013, 207: 191

[14] Leary R, Westwood A. Carbon, 2011, 49: 741

[15] Kamegawa T, Yamahana D, Yamashita H. J Phys Chem C, 2010, 114: 15049

[16] Wei W, Yu C, Zhao Q F, Li G S, Wan Y. Chem-Eur J, 2013, 19: 566

[17] Qian X F, Wang Z, Wan Y. J Colloid Interface Sci, 2009, 335: 222

[18] Wei W, Yu C, Zhao Q F, Qian X F, Li G S, Wan Y. Appl Catal B, DOI: 10.1016/j.apcatb.2013.04.048

[19] Feng C M, Li H X, Wan Y. J Nanosci Nanotechnol, 2009, 9: 1558

[20] Zhuang X, Wan Y, Feng C M, Shen Y, Zhao D Y. Chem Mater, 2009, 21: 706

[21] Tian B Z, Liu X Y, Tu B, Yu C Z, Fan J, Wang L M, Xie S H, Stucky G D, Zhao D Y. Nat Mater, 2003, 2: 159

[22] Ohsaka T, Izumi F, Fujiki Y. J Raman Spectrosc, 1978, 7: 321

[23] Shoute L C T, Loppnow G R. J Am Chem Soc, 2003, 125: 15636

[24] Parker J C, Siegel R W. Appl Phys Lett, 1990, 57: 943

[25] Zhang W F, He Y L, Zhang M S, Yin Z, Chen Q. J Phys D, 2000, 33: 912

[26] Zhang H R, Xie C F, Zhang Y F, Liu G S, Li Z H, Liu C Y, Ma X P, Zhang W F. J Appl Phys, 2008, 103: 103107

[27] Zhang Y, Zhang P, Huo Y N, Zhang D Q, Li G S, Li H X. Appl Catal B, 2012, 115-116: 236

[28] Zhang X Y, Li H P, Cui X L, Lin Y H. J Mater Chem, 2010, 20: 2801

[29] Ren W J, Ai Z H, Jia F L, Zhang L Z, Fan X X, Zou Z G. Appl Catal B, 2007, 69: 138

[30] Zhao L, Chen X F, Wang X C, Zhang Y J, Wei W, Sun Y H, Antonietti M, Titirici M M. Adv Mater, 2010, 22: 3317

[31] Velasco L F, Parra J B, Ania C O. Appl Surf Sci, 2010, 256: 5254

[32] Vijayan B K, Dimitrijevic N M, Finkelstein-Shapiro D, Wu J, Gray K A. ACS Catal, 2011, 2: 223

[33] Woan K, Pyrgiotakis G, Sigmund W. Adv Mater, 2009, 21: 2233

[34] Tseng Y H, Kuo C S, Huang C H, Li Y Y. Z Phys Chem, 2010, 224: 843

[35] Tauc J, Grigorovici R, Vancu A. Phys Status Solidi B, 1966, 15: 627

[36] Sun D G, Du J, Liu Z H, Tao C Y, Zhai J. Spectrosc Spect Anal (孙大贵, 杜军, 刘作华, 陶长元, 翟俊. 光谱学与光谱分析), 2011, 31: 525

[37] Xu Y J, Zhuang Y B, Fu X Z. J Phys Chem C, 2010, 114: 2669

[38] Cong Y, Li X K, Qin Y, Dong Z J, Yuan G M, Cui Z W, Lai X J. Appl Catal B, 2011, 107: 128

[39] Wu Z X, Webley P A, Zhao D Y. Langmuir, 2010, 26: 10277

[40] Kontos A I, Likodimos V, Stergiopoulos T, Tsoukleris D S, Falaras P, Rabias I, Papavassiliou G, Kim D, Kunze J, Schmuki P. Chem Mater, 2009, 21: 662

[41] Maeng Y J, Yoon B S, Suh M H, Im W B, Lee S H. Polym Compos, 2000, 21: 41

[42] Dong W Y, Sun Y J, Lee C W, Hua W M, Lu X C, Shi Y F, Zhang S C, Chen J M, Zhao D Y. J Am Chem Soc, 2007, 129: 13894

[43] Qian X F, Wan Y, Wen Y L, Jia N Q, Li H X, Zhao D Y. J Colloid Interface Sci, 2008, 328: 367

[44] Liu R L, Ren Y J, Shi Y F, Zhang F, Zhang L J, Tu B, Zhao D Y. Chem Mater, 2008, 20: 1140

[45] Chang P Y, Huang C H, Doong R A. Carbon, 2012, 50: 4259

[46] Li D L, Zhou H S, Honma I. Nat Mater, 2004, 3: 65

[47] Li Y F, Xu D H, Oh J I, Shen W Z, Li X, Yu Y. ACS Catal, 2012, 2: 391

[48] Chen D M, Jiang Z Y, Geng J Q, Wang Q, Yang D. Ind Eng Chem Res, 2007, 46: 2741

[49] Ania C O, Parra J B, Pis J J. Adsorpt Sci Technol, 2004, 22: 337

[50] Zhang Z H, Xu Y, Ma X P, Li F Y, Liu D N, Chen Z L, Zhang F Q, Dionysiou D D. J Hazard Mater, 2012, 209-210: 271

[51] Tseng R L, Tseng S K. J Colloid Interface Sci, 2005, 287: 428

[52] D?browski A, Podko?cielny P, Hubicki Z, Barczak M. Chemosphere, 2005, 58: 1049

[53] Terzyk A P. J Colloid Interface Sci, 2003, 268: 301