Effect of calcination temperature of Ni/SiO2-ZrO2 catalyst on its hydrodeoxygenation of guaiacol

doi:10.1016/S1872-2067(12)60733-5

Abstract

Abstract:

SiO₂-ZrO₂composites were synthesized by chemical precipitation and used to prepare a series of bifunctional Ni/SiO₂-ZrO₂ catalysts by impregnation. The effect of calcination temperature on the catalyst structure and its catalysis of the hydrodeoxygenation of guaiacol was investigated. Guaiacol was converted to cyclohexane by a synergism between the metal center and solid acid support. The catalyst calcined at 500℃ gave a maximum 100% guaiacol conversion and 96.8% selectivity for cyclohexane. The catalyst samples were characterized by N₂adsorption, H₂ chemisorption, X-ray diffraction, H₂ temperature-programmed reduction, NH₃ temperature-programmed desorption, and Raman spectroscopy. The synthesized SiO₂-ZrO₂ was an amorphous oxide. The Ni/SiO₂-ZrO₂ catalyst calcined at 500℃ has more acidity, smaller NiO particles, and larger BET surface area and pore volume, which gave it the best catalytic performance.

Key words: Nickel, Silica, Zirconia, Calcination temperature, Guaiacol, Hydrodeoxygenation, Cyclohexane

Xinghua Zhang, Qi Zhang, Lungang Chen, Ying Xu, Tiejun Wang, Longlong Ma. Effect of calcination temperature of Ni/SiO₂-ZrO₂ catalyst on its hydrodeoxygenation of guaiacol[J]. Chinese Journal of Catalysis, 2014, 35(3): 302-309.

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Effect of calcination temperature of Ni/SiO₂-ZrO₂ catalyst on its hydrodeoxygenation of guaiacol

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