Alcohol-treated SiO2 as the support of Ir-Re/SiO2 catalysts for glycerol hydrogenolysis

doi:10.1016/S1872-2067(16)62517-2

Chinese Journal of Catalysis ›› 2016, Vol. 37 ›› Issue (11): 2009-2017.DOI: 10.1016/S1872-2067(16)62517-2

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Alcohol-treated SiO₂ as the support of Ir-Re/SiO₂ catalysts for glycerol hydrogenolysis

Wenting Luo^a,c, Yuan Lyu^a, Leifeng Gong^a, Hong Du^a,c, Miao Jiang^a,c, Yunjie Ding^a,b

a Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;
b State Key Laboratory for Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;
c University of Chinese Academy of Sciences, Beijing 100049, China

Received:2016-07-25 Revised:2016-08-30 Online:2016-11-25 Published:2016-11-25
Contact: Yunjie Ding,Tel/Fax:+86-411-84379143; E-mail:dyj@dicp.ac.cn;Yuan Lyu,Tel/Fax:+86-411-84379143; E-mail:luyuan@dicp.ac.cn
Supported by:
This work was supported by the National Natural Science Foundation of China (21403217).

Abstract

Abstract:

The surface of SiO₂ support was pretreated by C1-C4 normal alcohols before the impregnation of iridium and rhenium precursors. These catalysts were applied in high concentration glycerol aque-ous solution hydrogenolysis. The catalysts prepared from the pretreated supports exhibited high catalytic activity because of the formation of more active sites from a high dispersion of iridium oxide and rhenium oxide. The catalysts with the support pretreated by 1-propanol showed the highest glycerol conversion of 59.5%. The supports and catalysts were characterized by FT-IR, ni-trogen adsorption, TPR, XRD, TEM, H₂-chemisorption and NH₃-TPD.

Key words: Glycerol hydrolysis, 1,3-Propanediol, Iridium, Rhenium, Alcohol pretreatment

Wenting Luo, Yuan Lyu, Leifeng Gong, Hong Du, Miao Jiang, Yunjie Ding. Alcohol-treated SiO₂ as the support of Ir-Re/SiO₂ catalysts for glycerol hydrogenolysis[J]. Chinese Journal of Catalysis, 2016, 37(11): 2009-2017.

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Alcohol-treated SiO₂ as the support of Ir-Re/SiO₂ catalysts for glycerol hydrogenolysis

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