Photoelectrocatalysis for high-value-added chemicals production

doi:10.1016/S1872-2067(21)63923-2

Chinese Journal of Catalysis ›› 2022, Vol. 43 ›› Issue (3): 595-610.DOI: 10.1016/S1872-2067(21)63923-2

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Photoelectrocatalysis for high-value-added chemicals production

Yucong Miao, Mingfei Shao^*()

State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing 100029, China

Received:2021-07-21 Revised:2021-07-21 Online:2022-03-18 Published:2022-02-18
Contact: Mingfei Shao
About author:Prof. Dr. Mingfei Shao (State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology (BUCT)) received his Ph.D degree in 2014 from Beijing University of Chemical Technology under the supervision of Prof. Xue Duan, after which he joined the staff of BUCT. He was also a visiting student at the University of Oxford in 2013. His research directions include intercalation chemistry and energy materials, electrocatalysis/photoelectrocatalysis and advanced energy devices. He has been published in more than 80 SCI papers as the first or corresponding/co-corresponding author in international journals such as J. Am. Chem. Soc, Angew. Chem. Int. Ed., Adv. Mater., Chem, which have been cited more than 7500 times (H index = 45). More than 10 Chinese patents have been authorized respect to his work. He proposed a new idea of photoelectronsyhthesis/electrosynthesis for the hydrogen generation coupled with organic oxidation. He also proposed a new method of integrated electrode design based on layered double hydroxides. He has obtained and award from the National Natural Science Foundation of China--Outstanding Youth Foundation in 2019, and Catalysis Rising Star Award from the Catalysis Society of China in 2021. He joined the editorial board of Chin. J. Catal. in 2020.
Supported by:
National Natural Science Foundation of China(2209003);National Natural Science Foundation of China(21922501);National Natural Science Foundation of China(21871021);National Natural Science Foundation of China(21521005);Beijing Natural Science Foundation(2192040)

Abstract

Abstract:

Photoelectrocatalysis (PEC) is a promising approach that can convert renewable solar energy into chemical energy, while most concern is concentrated on PEC water splitting to obtain high-value-added fuel—hydrogen. In practice, more economic benefits can be produced based on PEC technique, such as H₂O oxidative H₂O₂ synthesis, organic selective oxidation, organic pollutants degradation and CO₂ reduction. Although there are plenty of excellent reviews focusing on the PEC water splitting system, the production of various high-value-added chemicals in PEC systems has not been discussed synthetically. This Account will focus on the production process of various high-value-added chemicals through PEC technology. The photoelectrode design, reaction environment and working mechanisms of PEC systems are also discussed in detail. We believe that this comprehensive Account of the expanded application of photoelectrocatalysis can add an inestimable impetus to the follow-up development of this technology.

Key words: Photoelectrocatalysis, High-value-added chemicals, Photoelectrode, Organic oxidation, Carbon dioxide reduction

Yucong Miao, Mingfei Shao. Photoelectrocatalysis for high-value-added chemicals production[J]. Chinese Journal of Catalysis, 2022, 43(3): 595-610.

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Figures/Tables 13

Fig. 1. (a) The conversion of reactants required to achieve high-value-added chemicals production through photoelectrocatalysis; (b) The energy band structure of several common semiconductors and the redox potential [26-28].

Fig. 2. Schematic diagram of the reaction steps of overall water splitting and photoanode improvement strategies.

Fig. 3. (a) Schematic diagram of dye-sensitized TiO2/[CoFe-JG] electrode constructed by in-situ modification of Prussian blue analog on TiO2 photoanode. Reprinted with permission from Ref. [56]. Copyright 2020, John Wiley and Sons. (b) Au/UCN/TiO2 photoelectrode and its working mechanism of absorbing UV-vis-NIR light. Reprinted with permission from Ref. [59]. Copyright 2019, American Chemical Society. TEM (c) and HRTEM (d) images of Au/CdSe nanodumbbells; (e) Photocurrent stability of the Au/CdSe nanodumbbell photoanode at 0.4 V vs. RHE under light illumination at λ > 700 nm. (c?e) Reprinted with permission from Ref. [60]. Copyright 2019, John Wiley and Sons.

Fig. 4. (a) Separation of hole and charge during water oxidation of TiO2 photoelectrode. Adapted with permission from Ref. [43]. Copyright 2016, Royal Society of Chemistry. (b) Mechanism of water oxidation of MOs-[PDDA-Aux@GSH]n photoanode. (a,b) Reprinted with permission from Ref. [65]. Copyright 2020, American Chemical Society. (c) Schematic diagram of selective deposition of reduction and oxidation cocatalysts on different facets of BiVO4 with the help of the separation of electrons and holes; (d) SEM images of Pt/MnOx/BiVO4. (c,d) Reprinted with permission from Ref. [77]. Copyright 2014, Royal Society of Chemistry. (e)

Fig. 5. (a) Comparison of PEC and EC water oxidation processes to produce H2O2; (b) The path of each product and the thermodynamic trend in the water oxidation process.

Fig. 6. (a) Volcano plots of H2O2 production activity. Reprinted with permission from Ref. [83]. Copyright 2017, Springer Nature. (b) Yield of O2 and Faraday efficiency of O2 and H2O2 of BiVO4, SnO2/BiVO4 and SnO2-x/BiVO4 photoanodes; (c) Mechanism of suppression of OER by SnO2-x/BiVO4 photoanodes. (b,c) Reprinted with permission from Ref. [23]. Copyright 2020, American Chemical Society. (d) Diagram of free energy of BiVO4 (001) with or without oxygen vacancies. Reprinted with permission from Ref. [13]. Copyright 2021, John Wiley and Sons.

Fig. 7. Various reactions realized by PEC organic oxidation.

Fig. 8. (a) Table of TiO2/C photoanode oxidation of various aromatic alcohols; (b) Mechanism of oxidation of benzyl alcohol on TiO2/C photoanode. (a,b) Reprinted with permission from Ref. [15]. Copyright 2017, John Wiley and Sons. (c) Mass spectra of benzaldehyde obtained by oxidation of G@U-LDH@BVO photoanode in (I) H2O solution, (II) 10% H218O solution, (III) 80% H218O solution; (d) Article proposed mechanism of oxidation of benzyl alcohol to benzaldehyde by G@U-LDH@BVO photoanode. (c,d) Reprinted with permission from Ref. [87]. Copyright 2020, American Chemical Society.

Fig. 9. (a) Energy profile diagram of BiVO4 oxidized glycerol intermediates. Reprinted with permission from Ref. [92]. Copyright 2019, Springer Nature. (b) Diagram of the oxidation mechanism of HMF in a photoelectrocatalysis system using TEMPO as the medium. Reprinted with permission from Ref. [14]. Copyright 2015, Springer Nature. (c) Schematic illustration for different facets of WO3 nanobar arrays; (d) SEM images of WO3 nanobar arrays; (e) PEC oxidation process of methane. (c?e) Reprinted with permission from Ref. [90]. Copyright 2021, John Wiley and Sons.

Fig. 10. (a) Photocurrent-potential curves under illumination of SnO2@BiVO4/Co-Pi photoanode in 0.1M PBS with/without urea. Reprinted with permission from Ref. [88]. Copyright 2019, Royal Society of Chemistry. (b) Durability of F-BiVO4@NiFe-LDH photoanode for degradation of TCH. Reprinted with permission from Ref. [106]. Copyright 2020, Elsevier. (c) Photoelectrocatalytic CBZ oxidation couple with HER/CO2RR system. (d) Recycling test for CBZ degradation. (c,d) Reprinted with permission from Ref. [107]. Copyright 2021, Elsevier. (e) Schematic of the fabrication process of the (S)-DCPP-molecular-imprinted single-crystalline TiO2 photoelectrodes. Reprinted with permission from Ref. [100]. Copyright 2017, Elsevier. (f) Path of SnO2/010-BVO controlled conversion 2,4-DCP. Reprinted with permission from Ref. [108]. Copyright 2020, American Chemical Society.

Fig. 11. (a) Relaxation after CO2 adsorbed on AZO surface; (b) Calculation of free energy for different reduction paths of CO2. (a,b) Reprinted with permission from Ref. [119]. Copyright 2020, Elsevier. (c) Diagram of composite photocathode. Reprinted with permission from Ref. [121]. Copyright 2020, John Wiley and Sons. (d) Schematic mechanism of CoPcP for converting CO2 to CO. Reprinted with permission from Ref. [122]. Copyright 2021, American Chemical Society.

Fig. 12. (a) Diagram of the mechanism of the conversion of CO2 to methanol on the surface of Cu/Cu2O. Reprinted with permission from Ref. [117]. Copyright 2018, John Wiley and Sons.. (b) Adsorption behavior on g-C3N4/ZnTe heterojunction of CO2 (1) and CO (2); (c) Schematic diagram of g-C3N4/ZnTe heterojunction photocathode. (b,c) Reprinted with permission from Ref. [127]. Copyright 2019, Elsevier.

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Photoelectrocatalysis for high-value-added chemicals production

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