Unveiling the

doi:10.1016/S1872-2067(24)60028-8

Chinese Journal of Catalysis ›› 2024, Vol. 61: 37-53.DOI: 10.1016/S1872-2067(24)60028-8

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Unveiling the "sono-physico-chemical" essence: Cavitation and vibration effects in ultrasound-assisted processes

Wenyuan Liu^a, Jun Li^a, Zhuan Chen^a, Zhiyan Liang^a, Bo Yang^a, Kun Du^a, Jiangchen Fu^a, Ali Reza Mahjoub^b, Mingyang Xing^a^,^c^,^*()

^aKey Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Feringa Nobel Prize Scientist Joint Research Center, Frontiers Science Center for Materiobiology and Dynamic Chemistry, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, China
^bDepartment of Chemistry, Faculty of Basic Sciences, Tarbiat Modares University, Tehran, Iran
^cShanghai Engineering Research Center for Multi-media Environmental Catalysis and Resource Utilization, East China University of Science and Technology, Shanghai 200237, China

Received:2024-02-13 Accepted:2024-04-07 Online:2024-06-18 Published:2024-06-20
Contact: * E-mail: mingyangxing@ecust.edu.cn (M. Xing).
About author:Mingyang Xing (School of Chemistry and Molecular Engineering, East China University of Science and Technology) is the Professor, doctoral supervisor in the School of Chemistry and Molecular Engineering, East China University of Science and Technology (ECUST). He obtained his Doctoral Degree in 2012 from ECUST, and then worked at University of California, Riverside as a visiting scholar for one year. His research focuses on the design and preparation of functional nanomaterials and applications to the environmental fields, including (1) Enrichment and degradation of organic pollutants; (2) Recycling of organic wastewater: directed conversion of organic pollutants, hydrogen production of wastewater; (3) Seawater resource: seawater desalination, seawater hydrogen production, etc; (4) Resource of greenhouse gases. He has published more than 150 papers in SCI journals in these areas, which have been cited more than 15000 times (H-index: 68).
Supported by:
National Natural Science Foundation of China(22325602);National Natural Science Foundation of China(22176060);Program of Shanghai Academic/Technology Research Leader(23XD1421000)

Abstract

Abstract:

Ultrasound-assisted processes, widely applied in cleaning, synthesis, and catalysis, exhibit significant application potential, with their impact rooted in the interplay between ultrasound and the physicochemical properties of substances. Therefore, it is emphasized here to understand these processes through a "sono-physico-chemical" angle for a deeper comprehension of reaction mechanisms and broader application. Highlighting cavitation and vibration effects, the ultrasound-assisted chemistry processes are categorized. Cavitation is emphasized for pollutant degradation, while vibration is primarily applied for inducing the piezoelectric effect. Additionally, points that are easy to be ignored in the current ultrasonic assisted catalysis process are proposed, such as synergistic index calculations, cost assessments, etc. Furthermore, the latest innovative application of ultrasonic assisted process in wastewater recycling is introduced. Finally, the review advocates for the future integration of ultrasound-assisted processes into new catalytic processes or application scenarios.

Key words: Ultrasonic assisted process, Cavitation effect, Vibration effect, Piezoelectric effect, Pollutant degradation

Wenyuan Liu, Jun Li, Zhuan Chen, Zhiyan Liang, Bo Yang, Kun Du, Jiangchen Fu, Ali Reza Mahjoub, Mingyang Xing. Unveiling the "sono-physico-chemical" essence: Cavitation and vibration effects in ultrasound-assisted processes[J]. Chinese Journal of Catalysis, 2024, 61: 37-53.

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Figures/Tables 10

Fig. 1. The results of searching the term "ultrasound assisted" on the Web of Science related to chemistry.

Fig. 2. Comprehension ultrasound-assisted processes in the view of "sono-physico-chemical".

Fig. 3. (a) Ultrasonic cavitation effect during propagation of ultrasonic wave. (b) Physical and chemical changes caused by cavitation effect.

Fig. 4. Principle (a) and application (b) of piezoelectric effect. (c) The application of cavitation and vibration effects in ultrasound-assisted processes. Reprinted with permission from Ref. [11]. Copyright 2011, WILEY-VCH. Reprinted with permission from Ref. [6]. Copyright 2020, Elsevier. Reprinted with permission from Ref. [10]. Copyright 2020, WILEY-VCH. Reprinted with permission from Ref. [24]. Copyright 2016, WILEY-VCH. Reprinted with permission from Ref. [12]. Copyright 2023, PNAS. Reprinted with permission from Ref. [13]. Copyright 2023, WILEY-VCH.

Fig. 5. (a) EPR spectra of defects in CoS2-com and CoS2-x at room temperature. (b) Long-term degradation of RhB in the CuPx (1 g L?1) system, the CoS2-1.5h (1 g L?1) system, the CoS2-1.5h (1 g L?1)/Fe3+ (0.1 g L?1) system and the CoS2-1.5h (1 g L?1)/Fe2+ (0.1 g L?1) system, respectively. (c) The mechanism of ROS generation and Fe ion circulation in the CoS2-1.5h system (red sphere: Co; white sphere: S; blue sphere: defect). Reprinted with permission from Ref. [10]. Copyright 2020, WILEY-VCH.

Fig. 6. (a) The reaction mechanism of the bubble cavity. Reprinted with permission from Ref. [68]. Copyright 2009, Elsevier. (b) Oxidation mechanism of oxidants in the US-oxidant systems. Reprinted with permission from Ref. [57]. Copyright 2023, Elsevier. (c) ARAC degradation kinetics, and corresponding pseudo-first order rate constant. Reprinted with permission from Ref. [58]. Copyright 2022, Elsevier. (d) Production of 7-hydroxycoumarin by bubble type and ultrasonic. (e) The reaction mechanism of nanobubble with ultrasonic cavitation. Reprinted with permission from Ref. [24]. Copyright 2023, Elsevier. (f) Proposed reaction schemes for degradation of organic matters by MgO@Z/UV/US system. (g) Comparison of different possible processes for the degradation of textile industrial effluent. Reprinted with permission from Ref. [69]. Copyright 2018, Elsevier. (h) Reaction mechanism of SEF process. Reprinted with permission from Ref. [64]. Copyright 2022, American Chemical Society.

Fig. 7. (a) Removal rate of HA and (b) removal kinetics of HA in a different reaction system. Reprinted with permission from Ref. [74]. Copyright 2021, Elsevier. (c) Effect of pH on the Malathion degradation. Reprinted with permission from Ref. [54]. Copyright 2021, Elsevier. (d) The performance of various processes in the intrinsic viscosity removal and COD removal from HPG. Reprinted with permission from Ref. [75]. Copyright 2023, Elsevier. (e) The cost ($) of removing 1 kg Malathion in different systems. Reprinted with permission from Ref. [54]. Copyright 2021, Elsevier. (f) Calculations of wastewater treatment cost for complete degradation of sulfide ions by cavitation processes combined with AOPs. Reprinted with permission from Ref. [76]. Copyright 2021, Elsevier. (g) Diagram of a photovoltaic PV system. Reprinted with permission from Ref. [78]. Copyright 2018, Elsevier. (h) Calorimetric energy efficiencies for different frequency and power settings. Reprinted with permission from Ref. [83]. Copyright 2023, Elsevier. (i) Comparison of pseudo-first-order removal rate constants (min-1) of PFASs observed in the 700 kHz, 250 W open system (Pd = 1250 W L-1) for the 24Mix-spiked deionized water, low TDS groundwater, and high TDS groundwater. Reprinted with permission from Ref. [84]. Copyright 2021, Elsevier.

Fig. 8. (a) Rate of H2 production of piezo-photocatalysis coupling activity. (b) Schematic diagram of piezo-photocatalysis for PbTiO3/CdS composites. Reprinted with permission from Ref. [91]. Copyright 2020, Elsevier. (c) 1O2 trapped by TEMP under different conditions. (d) Schematic diagram of the separation and migration of electron-hole pairs in pure BTO NCs with (left) and without (right) piezotronic effect. (e) Schematic diagram of the separation and migration of electron-hole pairs in Cu2-xO-BTO NCs with a piezotronic effect. Reprinted with permission from Ref. [88]. Copyright 2022, American Chemical Society. (f) Schematic diagram of band tilting of BTO-T under applied strain by laser-triggered micro-pressure and the corresponding piezo-catalytic reaction. Reprinted with permission from Ref. [92]. Copyright 2020, WILEY-VCH. (g) Structural changes and (h) difference charge density of SnS after applying compress (charge accumulation is in red and depletion in blue) (Green: Sn, Yellow: S). (i) Calculated DOS of SnS. Reprinted with permission from Ref. [25]. Copyright 2023, WILEY-VCH.

Fig. 9. (a) Schematic diagram of piezoelectricity coupling AOPs for H2 production from wastewater remediation. (b) The piezocatalytic H2 production rates of MoS2/Fe0 in solutions with different concentrations of NB. (c) The piezocatalytic H2 yield curves of MoS2/Fe0, MoS2/Fe0/PMS and MoS2/Fe0 (pH = 2.5) in NB solution. (d) The removal rates of TOC under different conditions. (e) Adsorption energy of different models. (f) Reaction energy in different pathways determined from the results of DFT. (g) The H2 yields of MoS2/Fe0/PMS piezocatalytic H2 production from actual soil remediation wastewater. Reprinted with permission from Ref. [12]. Copyright 2023, PNAS. (h) CO evolution of Co3S4/MoS2/PMS/US system under different conditions and (i) compared with homogeneous Fenton. (j) Calculated free energy diagram corresponding to the reaction path followed by carbonate conversion on the MoS2 and Co3S4/MoS2 catalysts. (k) Schematic diagram of selective production of CO from organic pollutants by piezocatalysis coupling AOPs. Reprinted with permission from Ref. [13]. Copyright 2023, WILEY-VCH.

Fig. 10. The development and important event of piezoelectric in catalysis. Reprinted with permission from Ref. [31] Copyright 2006, The American Association for the Advancement of Science. Reprinted with permission from Ref. [32]. Copyright 2010, Elsevier. Reprinted with permission from Ref. [107]. Copyright 2012, American Chemical Society. Reprinted with permission from Ref. [106]. Copyright 2012, Elsevier. Reprinted with permission from Ref. [110]. Copyright 2014, Macmillan Publishers Limited. Reprinted with permission from Ref. [26]. Copyright 2016, WILEY-VCH. Reprinted with permission from Ref. [111]. Copyright 2017, Elsevier. Reprinted with permission from Ref. [99]. Copyright 2020, WILEY-VCH. Reprinted with permission from Ref. [12]. Copyright 2023, PNAS. Reprinted with permission from Ref. [13]. Copyright 2023, WILEY-VCH.

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Unveiling the "sono-physico-chemical" essence: Cavitation and vibration effects in ultrasound-assisted processes

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