Effect of photon irradiation on the adsorption of CO2 on polycrystalline Cu

doi:10.1016/S1872-2067(12)60538-5

Abstract

Abstract:

The adsorption and photochemistry of CO₂ on ordered/disordered Cu surfaces were investigated using X-ray photoelectron and high resolution electron loss technique. Physisorbed CO₂ and chemisorbed CO₂^δ- species were isolated on different faces. Studies on the photochemical behavior of physisorbed and chemisorbed species were conducted with 193 nm laser irradiation. No photoinduced reaction occurred with the physisorbed species. Photoinduced dissociation was seen with chemisorbed species.

Key words: Carbon dioxide, Copper surface, Chemical adsorption, Photoinduced dissociation

WANG Shuai, XU Guoqin. Effect of photon irradiation on the adsorption of CO₂ on polycrystalline Cu[J]. Chinese Journal of Catalysis, 2013, 34(5): 865-870.

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References

[1] Song C S. Catal Today, 2006, 115: 2

[2] Chueh W C, Falter C, Abbott M, Scipio D, Furler P, Haile S M, Steinfeld A. Science, 2010, 330: 1797

[3] Ma J,Sun N N, Zhang X L, Zhao N, Xiao F K, Wei W, Sun Y H. Catal Today, 2009, 148: 221

[4] Wang D J, Tao F R, Zhao H H, Song H L, Chou L J. Chin J Catal (王丹君, 陶芙容, 赵华华, 宋焕玲, 丑玲军. 催化学报), 2011, 32: 1452

[5] Hirano K, Inoue K,Yatsu T. J Photochem Photobiol A, 1992, 64: 255

[6] Inoue T, Fujishima A, Konishi S, Honda K. Nature, 1979, 277: 637

[7] Jorgensen M E, Godowski P J, Onsgaard J. Proceedings of the 18th International Seminar on Surface Physics, 1997, 48: 299

[8] Rasmussen P B, Taylor P A,Chorkendorff I. Surf Sci, 1992, 270: 352

[9] Ernst K H, Schlatterbeck D, Christmann K. Phys Chem Chem Phys, 1999, 1: 4105

[10] Christiansen M, Thomsen E V, Onsgaad J. Surf Sci, 1992, 261: 179

[11] Hadden R A, Vandervell, H D, Waugh K C, Webb G. Catal Lett, 1988, 1: 27

[12] Copperthwaite R G, Davies P R, Morris M A, Roberts M W, Ryder R A. Catal Lett, 1988, 1: 11

[13] Campbell C T, Daube K A, White J M. Surf Sci, 1987, 182: 458

[14] Krause J, Borgmann D,Wedler G. Surf Sci, 1996, 347: 1

[15] Chorkendorf I,Rasmussen P B. Surf Sci, 1992, 248: 35

[16] Pohl M, Otto A. Surf Sci, 1998, 406: 125

[17] Fu S S, Somorjai G A. Surf Sci, 1992, 262: 68

[18] Akemann W, Otto A. Surf Sci, 1993, 287-288: 104

[19] Akemann W, Otto A. Surf Sci, 1992, 272: 211

[20] Bartos B, Freund H J,Kuhlenbeck H,Neumann M, Lindner H, Muller K. Surf Sci, 1987, 179: 59

[21] Wambach J, Illing G, Freund H J. Chem Phys Lett, 1991, 184: 239

[22] Chen L, Magtoto N, Ekstrom B, Kelber J. Thin Solid Films, 2000, 376: 115

[23] Akemann W, Raman J, Otto A. Spectrosc, 1991, 22: 797

[24] Albano E V, Daiser S, Miranda R, Wandelt K. Surf Sci, 1986, 150: 367

[25] Elckmans J, Otto A, Goldman A. Surf Sci, 1986, 171: 415

[26] McCash E M. Surface Chemistry. USA: Oxford University Press 2001

[27] Freund H J, Roberts M W. Surf Sci Reports, 1996, 25: 225

[28] Freund H J, Messmer R P. Surf Sci, 1986, 172: 1

[29] Lehwald S, Rocca M, Ibach H, Rahman T S. J Electron Spectrosc, 1986, 38: 29

[30] Illing G, Heskett D, Plummer E W, Freund H J, Somers J, Linder Th,Bradshaw A M, Buskotte U, Neumann M, Starke U, Heinz K, De Andres P L, Saldin D, Pendry J B. Surf Sci, 1988, 206: 1

[31] Okabe H. Photochemistry of Small Molecules. New York: Wiley. 1978

[32] Sueyoshi T, Sasaki T, Iwasawa Y. Surf Sci, 1995, 343: 1

[33] Deng X Y, Verdaguer A, Herranz T, Weis C, Bluhm H, Salmeron M. Langmuir, 2008, 24: 9474

Effect of photon irradiation on the adsorption of CO₂ on polycrystalline Cu

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