CO oxidation over Au/ZrLa-doped CeO2 catalysts: Synergistic effect of zirconium and lanthanum

doi:10.1016/S1872-2067(15)61113-5

Abstract

Abstract:

The physicochemical properties of nanosized Au catalysts supported on doped CeO₂ and their catalytic performance for the CO oxidation reaction were investigated. The Au/Zr-doped CeO₂ catalyst is much more active than undoped Au/CeO₂, while Au/ZrLa-doped CeO₂ shows the highest activity. Characterization of the catalysts by X-ray diffraction, transmission electron microscopy (TEM), high-resolution TEM, and the X-ray absorption fine structure technique shows high homogeneity of the oxide supports and well-dispersed nanosized Au nanoparticles. Raman spectroscopy, X-ray photoelectron spectroscopy, and H₂-tempeature-programmed reduction show that the surface oxygen species are the main factor for the catalytic activity in the CO oxidation reaction, while the supported Au species can improve the redox properties and create oxygen vacancy sites on the support. The oxidation state of Au is not the main factor governing the activity of Au/doped-CeO₂ catalysts. Additionally, the synergistic effect of Zr and La is discussed.

Key words: Gold catalyst, Doped ceria, Oxygen vacancy, Carbon monoxide oxidation, Metal-support interaction

Qi Yang, Linying Du, Xu Wang, Chunjiang Jia, Rui Si . CO oxidation over Au/ZrLa-doped CeO₂ catalysts: Synergistic effect of zirconium and lanthanum[J]. Chinese Journal of Catalysis, 2016, 37(8): 1331-1339.

×
share this article

Add to citation manager EndNote|Ris|BibTeX

URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(15)61113-5

https://www.cjcatal.com/EN/Y2016/V37/I8/1331

References

[1] Y. Guo, D. Gu, Z. Jin, P. P. Du, R. Si, J. Tao, W. Q. Xu, Y. Y. Huang, S. Senanayake, Q. S. Song, C. J. Jia, F. Schüth, Nanoscale, 2015, 7, 4920-4928.
[2] L. Li, H. Li, X. C. Zeng, Chem. Commun., 2015, 51, 9535-9538.
[3] I. X. Green, W. J. Tang, M. Neurock, J. T. Yates Jr., Science, 2011, 333, 736-739.
[4] J. Ke, W. Zhu, Y. Y. Jiang, R. Si, Y. J. Wang, S. C. Li, C. H. Jin, H. C. Liu, W. G. Song, C. H. Yan, Y. W. Zhang, ACS Catal., 2015, 5, 5164-5173.
[5] Q. Fu, A. Weber, M. Flytzani-Stephanopoulos, Catal. Lett., 2001, 77, 87-95.
[6] D. Gu, C. J. Jia, C. Weidenthaler, H. J. Bongard, B. Splietho, W. Schmidt, F. Schuth, J. Am. Chem. Soc., 2015, 137, 11407-11418.
[7] K. T. Højholt, A. B. Laursen, S. Kegnæs, C. H. Christensen, Top. Catal., 2011, 54, 1026-1033.
[8] A. A. Herzing, C. J. Kiely, A. F. Carley, P. London, G. T. Hutchings, Science, 2008, 321, 1331-1335.
[9] G. C. Bond, D. T. Thompson, Gold Bull., 2000, 33, 41-50.
[10] N. Weiher, E. Bus, L. Delannoy, C. Louis, D. E. Ramaker, J. T. Miller, J. A. van Bokhoven, J. Catal., 2006, 240, 100-107.
[11] G. J. Hutchings, M. S. Hall, A. F. Carley, P. Landon, B. E. Solsona, C. J. Kiely, A. Herzing, M. Makkee, J. A. Moulijn, A. Overweg, J. C. Fierro-Gonzalez, J. Guzman, B. C. Gates, J. Catal., 2006, 242, 71-81.
[12] G. Avgouropoulos, M. Manzoli, F. Boccuzzi, T. Tabakova, J. Papavasiliou, T. Ioannides, V. Idakiev, J. Catal., 2008, 256, 237-247.
[13] M. M. Schubert, S. Hackenberg, A. C. van Veen, M. Muhler, V. Plzak, R. Jürgen Behm, J. Catal., 2001, 197, 113-122.
[14] M. Nolan, V. S. Verdugo, H. Metiu, Surf. Sci., 2008, 602, 2734-2742.
[15] D. Widmann, R. Leppelt, R. J. Behm, J. Catal., 2007, 251, 437-442.
[16] Y. Chen, P. Hu, M. H. Lee, H. F. Wang, Surf. Sci., 2008, 602, 1736-1741.
[17] N. Ta, J. Y. Li, S. Chenna, P. A. Crozier, Y. Li, A. L. Chen, W. J. Shen, J. Am. Chem. Soc., 2012, 134, 20585-20588.
[18] J. Ke, J. W. Xiao, W. Zhu, H. C. Liu, R. Si, Y. W. Zhang, C. H. Yan, J. Am. Chem. Soc., 2013, 135, 15191-15200.
[19] W. W. Wang, P. P. Du, S. H. Zou, H. Y. He, R. X. Wang, Z. Jin, S. Shi, Y. Y. Huang, R. Si, Q. S. Song, C. J. Jia, C. H. Yan, ACS Catal., 2015, 5, 2088-2099.
[20] S. Carrettin, P. Concepción, A. Corma, J. M. López Nieto, V. F. Puntes, Angew. Chem. Int. Ed., 2004, 43, 2538-2540.
[21] J. Guzman, S. Carrettin, A. Corma, J. Am. Chem. Soc., 2005, 127, 3286-3287.
[22] R. Si, Y. W. Zhang, L. M. Wang, S. J. Li, B. X. Lin, W. S. Chu, Z. Y. Wu, C. H. Yan, J. Phys. Chem. C, 2007, 111, 787-794.
[23] A. A. Fonseca, J. M. Fisher, D. Ozkaya, M. D. Shannon, D. Thompsett, Top. Catal., 2007, 44, 223-235.
[24] Q. Fu, H. Saltsburg, M. Flytzani-Stephanopoulo, Science, 2003, 301, 935-938.
[25] R. Si, Y. W. Zhang, S. J. Li, B. X. Lin, C. H. Yan, J. Phys. Chem. B, 2004, 108, 12481-12488.
[26] J. S. Moura , J. da Silva Lima Fonseca, N. Bion, F. Epron, T. de Freitas Silvac, C. G. Maciel, J. M. Assaf, M. do Carmo Rangel, Catal. Today, 2014, 228, 40-50.
[27] Q. Wang, X. H. Li, W. Y. Li, J. Feng, Catal. Commun., 2014, 50, 21-24.
[28] M. Yashima, H. Arashi, M. Kakihana, M. Yoshimura, J. Am. Cream. Soc., 1994, 77, 1067-1071.
[29] K. Z. Li, H. Wang, Y. G. Wei, D. X. Yan, Appl. Catal. B, 2010, 97, 361-372.
[30] Q. Yang, M. Kong, Z. Y. Fan, X. J. Meng, J. H. Fei, F. S. Xiao, Energy Fuels, 2012, 26, 4475-4480.
[31] P. Bera, M. S. Hegde, Catal. Lett., 2002, 79, 75-81.
[32] X. S. Huang, H. Sun, L. C. Wang, Y. M. Liu, K. N. Fan, Y. Cao, Appl. Catal. B, 2009, 90, 224-232.
[33] A. M. Venezia, G. Pantaleo, A. Longo, G. Di Carlo, M. P. Casaletto, F. L. Liotta, G. Deganello, J. Phys. Chem. B, 2005, 109, 2821-2827.
[34] F. Morfin, A. Ait-Chaou, M. Lomello, J. L. Rousset, J. Catal., 2015, 331, 210-216.
[35] W. L. Deng, A. I. Frenkel, R. Si, M. Flytzani-Stephanopoulos, J. Phys. Chem. C, 2008, 112, 12834-12840.
[36] A. I. Frenkel, C. W. Hills, R. G. Nuzzo, J. Phys. Chem. B, 2001, 105, 12689-12703.
[37] R. Si, M. Flytzani-Stephanopoulos, Angew. Chem. Int. Ed., 2008, 47, 2884-2887.
[38] S. Zhang, X. S. Li, B. B. Chen, X. B. Zhu, C. Shi, A. M. Zhu, ACS Catal., 2014, 4, 3481-3489.
[39] H. G. Peng, Y. Peng, X. L. Xu, X. Z. Fang, Y. Liu, J. X. Cai, X. Wang, Chin. J. Catal., 2015, 36, 2004-2010.
[40] L. Jiang, H. W. Zhu, R. Razzaq, M. L. Zhu, C. S. Li, Z. X. Li, Int. J. Hydrogen Energy, 2012, 37, 15914-15924.

CO oxidation over Au/ZrLa-doped CeO₂ catalysts: Synergistic effect of zirconium and lanthanum

PDF (PC)

Knowledge

Abstract

Cite this article

share this article

share this article

References

Related Articles 15

Recommended Articles

Metrics

[1]	Mingjie Cai, Yanping Liu, Kexin Dong, Xiaobo Chen, Shijie Li. Floatable S-scheme Bi₂WO₆/C₃N₄/carbon fiber cloth composite photocatalyst for efficient water decontamination [J]. Chinese Journal of Catalysis, 2023, 52(9): 239-251.
[2]	Haifeng Liu, Xiang Huang, Jiazang Chen. Surface electronic state modulation promotes photoinduced aggregation and oxidation of trace CO for lossless purification of H₂ stream [J]. Chinese Journal of Catalysis, 2023, 51(8): 49-54.
[3]	Xiu-Qing Qiao, Chen Li, Zizhao Wang, Dongfang Hou, Dong-Sheng Li. TiO_2-_x@C/MoO₂Schottky junction: Rational design and efficient charge separation for promoted photocatalytic performance [J]. Chinese Journal of Catalysis, 2023, 51(8): 66-79.
[4]	Fengwei Zhang, Hefang Guo, Mengmeng Liu, Yang Zhao, Feng Hong, Jingjing Li, Zhengping Dong, Botao Qiao. Enhancing the chemoselective hydrogenation of nitroarenes: Designing a novel surface-strained carbon-based Pt nanocatalyst [J]. Chinese Journal of Catalysis, 2023, 48(5): 195-204.
[5]	Yan Zeng, Hui Wang, Huiru Yang, Chao Juan, Dan Li, Xiaodong Wen, Fan Zhang, Ji-Jun Zou, Chong Peng, Changwei Hu. Ni nanoparticle coupled surface oxygen vacancies for efficient synergistic conversion of palmitic acid into alkanes [J]. Chinese Journal of Catalysis, 2023, 47(4): 229-242.
[6]	Zhijie Zhang, Xuesheng Wang, Huiling Tang, Deben Li, Jiayue Xu. Modulation of Fermi level gap and internal electric field over Cs₃Bi₂Br₉@V_O-In₂O₃S-scheme heterojunction for boosted charge separation and CO₂ photoconversion [J]. Chinese Journal of Catalysis, 2023, 55(12): 227-240.
[7]	Tingting Jiang, Weiwei Xie, Shipeng Geng, Ruchun Li, Shuqin Song, Yi Wang. Constructing oxygen vacancy-regulated cobalt molybdate nanoflakes for efficient oxygen evolution reaction catalysis [J]. Chinese Journal of Catalysis, 2022, 43(9): 2434-2442.
[8]	Huayang Zhang, Wenjie Tian, Xiaoguang Duan, Hongqi Sun, Yingping Huang, Yanfen Fang, Shaobin Wang. Single-atom catalysts on metal-based supports for solar photoreduction catalysis [J]. Chinese Journal of Catalysis, 2022, 43(9): 2301-2315.
[9]	Xianwen Zhang, Zheng Li, Taifeng Liu, Mingrun Li, Chaobin Zeng, Hiroaki Matsumoto, Hongxian Han. Water oxidation sites located at the interface of Pt/SrTiO₃ for photocatalytic overall water splitting [J]. Chinese Journal of Catalysis, 2022, 43(8): 2223-2230.
[10]	Qing Yao, Jiabo Le, Shize Yang, Jun Cheng, Qi Shao, Xiaoqing Huang. A trace of Pt can significantly boost RuO₂ for acidic water splitting [J]. Chinese Journal of Catalysis, 2022, 43(6): 1493-1501.
[11]	Peng Li, Guoqiang Zhao, Ningyan Cheng, Lixue Xia, Xiaoning Li, Yaping Chen, Mengmeng Lao, Zhenxiang Cheng, Yan Zhao, Xun Xu, Yinzhu Jiang, Hongge Pan, Shi Xue Dou, Wenping Sun. Toward enhanced alkaline hydrogen electrocatalysis with transition metal-functionalized nitrogen-doped carbon supports [J]. Chinese Journal of Catalysis, 2022, 43(5): 1351-1359.
[12]	Yu Deng, Jue Li, Rumeng Zhang, Chunqiu Han, Yi Chen, Ying Zhou, Wei Liu, Po Keung Wong, Liqun Ye. Solar-energy-driven photothermal catalytic C-C coupling from CO₂ reduction over WO_3-_x [J]. Chinese Journal of Catalysis, 2022, 43(5): 1230-1237.
[13]	Xuemei Jia, Zichen Shen, Qiaofeng Han, Huiping Bi. Rod-like Bi₄O₅I₂/Bi₄O₅Br₂ step-scheme heterostructure with oxygen vacancies synthesized by calcining the solid solution containing organic group [J]. Chinese Journal of Catalysis, 2022, 43(2): 288-302.
[14]	Ke Wang, Shihui He, Yunzhi Lin, Xun Chen, Wenxin Dai, Xianzhi Fu. Photo-enhanced thermal catalytic CO₂ methanation activity and stability over oxygen-deficient Ru/TiO₂ with exposed TiO₂ {001} facets: Adjusting photogenerated electron behaviors by metal-support interactions [J]. Chinese Journal of Catalysis, 2022, 43(2): 391-402.
[15]	Shijie Li, Mingjie Cai, Yanping Liu, Chunchun Wang, Kangle Lv, Xiaobo Chen. S-Scheme photocatalyst TaON/Bi₂WO₆ nanofibers with oxygen vacancies for efficient abatement of antibiotics and Cr(VI): Intermediate eco-toxicity analysis and mechanistic insights [J]. Chinese Journal of Catalysis, 2022, 43(10): 2652-2664.