Significant role of carbonate radicals in tetracycline hydrochloride degradation based on solar light-driven TiO2-seashell composites: Removal and transformation pathways

doi:10.1016/S1872-2067(19)63525-4

Abstract

Abstract: TiO₂-seashell composites prepared via a sol-gel method were used to generate carbonate radicals (·CO₃^-) under solar light irradiation.·CO₃^-, a selective radical, was employed to degrade the target tetracycline hydrochloride contaminant. A series of characterizations was carried out to study the structure and composition of the synthesized TiO₂-seashell composite. This material exhibits excellent solar light-driven photochemical activity in the decomposition of tetracycline hydrochloride. The possible pathway and mechanism for the photodegradation process were proposed on the basis of high-resolution electrospray ionization time-of-flight mass spectrometry experiments. Finally, we investigated the reusability of the TiO₂-seashell composite. This study is expected to provide a new facile pathway for the application of·CO₃^- radicals to degrade special organic pollutants in water.

Key words: TiO₂-seashell, Carbonate radical, Photochemistry, Tetracycline hydrochloride, Mechanism

Jiaqi Wang, Qingrong Qian, Qinghua Chen, Xin-Ping Liu, Yongjin Luo, Hun Xue, Zhaohui Li. Significant role of carbonate radicals in tetracycline hydrochloride degradation based on solar light-driven TiO₂-seashell composites: Removal and transformation pathways[J]. Chinese Journal of Catalysis, 2020, 41(10): 1511-1521.

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Significant role of carbonate radicals in tetracycline hydrochloride degradation based on solar light-driven TiO₂-seashell composites: Removal and transformation pathways

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