Visible light-induced Z-scheme V2O5/g-C3N4 heterojunction catalyzed cascade reaction of unactivated alkenes

doi:10.1016/S1872-2067(22)64162-7

Abstract

Qing-Wen Gui, Fan Teng, Peng Yu, Yi-Fan Wu, Zhi-Bin Nong, Long-Xi Yang, Xiang Chen, Tian-Bao Yang, Wei-Min He. Visible light-induced Z-scheme V₂O₅/g-C₃N₄ heterojunction catalyzed cascade reaction of unactivated alkenes[J]. Chinese Journal of Catalysis, 2023, 44: 111-116.

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References

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Entry	Photocatalyst	Solvent	Yield (%)
1	g-C₃N₄	2-MeTHF	69
2	g-C₃N₄	EtOAc	22
3	g-C₃N₄	EtOH	trace
4	g-C₃N₄	DMC	trace
5	g-C₃N₄	H₂O	17
6	g-C₃N₄	Acetone	trace
7	g-C₃N₄	DCE	4
8	g-C₃N₄	MeCN	7
9	g-C₃N₄	DMF	trace
10	g-C₃N₄	DMSO	25
11	g-C₃N₄	THF	51
12	V₂O₅/g-C₃N₄	2-MeTHF	83
13	V₂O₅	2-MeTHF	22
14	TiO₂	2-MeTHF	N.R.
15	BiVO₄	2-MeTHF	N.R.
16	CdS	2-MeTHF	N.R.
17	fac-[Ir(ppy)₃] (5 mol%)	2-MeTHF	7
18	Ru(bpy)₃Cl₂·6H₂O (5 mol%)	2-MeTHF	trace
19	Mes-Acr⁺ClO₄^‒(5 mol%)	2-MeTHF	12
20	Rhodamine 6G (5 mol %)	2-MeTHF	5
21	Rhodamine B (5 mol %)	2-MeTHF	10
22^c	V₂O₅/g-C₃N₄	2-MeTHF	53
23^d	V₂O₅/g-C₃N₄	2-MeTHF	46
24^e	—	2-MeTHF	trace
25^f	V₂O₅/g-C₃N₄	2-MeTHF	N.R.
26^g	V₂O₅/g-C₃N₄	2-MeTHF	N.R.
27^h	V₂O₅/g-C₃N₄	2-MeTHF	29

Entry	Photocatalyst	Solvent	Yield (%)
1	g-C₃N₄	2-MeTHF	69
2	g-C₃N₄	EtOAc	22
3	g-C₃N₄	EtOH	trace
4	g-C₃N₄	DMC	trace
5	g-C₃N₄	H₂O	17
6	g-C₃N₄	Acetone	trace
7	g-C₃N₄	DCE	4
8	g-C₃N₄	MeCN	7
9	g-C₃N₄	DMF	trace
10	g-C₃N₄	DMSO	25
11	g-C₃N₄	THF	51
12	V₂O₅/g-C₃N₄	2-MeTHF	83
13	V₂O₅	2-MeTHF	22
14	TiO₂	2-MeTHF	N.R.
15	BiVO₄	2-MeTHF	N.R.
16	CdS	2-MeTHF	N.R.
17	fac-[Ir(ppy)₃] (5 mol%)	2-MeTHF	7
18	Ru(bpy)₃Cl₂·6H₂O (5 mol%)	2-MeTHF	trace
19	Mes-Acr⁺ClO₄^‒(5 mol%)	2-MeTHF	12
20	Rhodamine 6G (5 mol %)	2-MeTHF	5
21	Rhodamine B (5 mol %)	2-MeTHF	10
22^c	V₂O₅/g-C₃N₄	2-MeTHF	53
23^d	V₂O₅/g-C₃N₄	2-MeTHF	46
24^e	—	2-MeTHF	trace
25^f	V₂O₅/g-C₃N₄	2-MeTHF	N.R.
26^g	V₂O₅/g-C₃N₄	2-MeTHF	N.R.
27^h	V₂O₅/g-C₃N₄	2-MeTHF	29

Visible light-induced Z-scheme V₂O₅/g-C₃N₄ heterojunction catalyzed cascade reaction of unactivated alkenes

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