Construction of an operando dual-beam fourier transform infrared spectrometer and its application in the observation of isobutene reactions over nano-sized HZSM-5 zeolite

doi:10.1016/S1872-2067(17)62751-7

Chinese Journal of Catalysis ›› 2017, Vol. 38 ›› Issue (1): 13-19.DOI: 10.1016/S1872-2067(17)62751-7

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Construction of an operando dual-beam fourier transform infrared spectrometer and its application in the observation of isobutene reactions over nano-sized HZSM-5 zeolite

Jiaxu Liu^a, Jilei Wang^a, Wei Zhou^a, Cuilan Miao^a, Guang Xiong^a, Qin Xin^b, Hongchen Guo^a

a Department of Catalytic Chemistry and Engineering & State Key Laboratory of Fine Chemicals, Dalian University of Technology, Dalian 116012, Liaoning, China;
b State Key Laboratory for Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China

Received:2016-11-18 Revised:2016-12-08 Online:2017-01-18 Published:2017-01-18
Contact: Hongchen Guo,Tel/Fax:+86-411-84986120;E-mail:hongchenguo@163.com
Supported by:
This work was supported by the National Natural Science Foundation of China (21603023), and the PetroChina Innovation Foundation, China (2014D-5006-0501).

Abstract

Abstract:

An operando dual-beam Fourier transform infrared (DB-FTIR) spectrometer was successfully de-veloped using a facile method. The DB-FTIR spectrometer is suitable for the real-time study of the dynamic surface processes involved in gas/solid heterogeneous catalysis under real reaction condi-tions because it can simultaneously collect reference and sample spectra. The influence of gas-phase molecular vibration and heat irradiation at real reaction temperatures can therefore be eliminated. The DB-FTIR spectrometer was successfully used to follow the transformation of isobutene over nano-sized HZSM-5 zeolite under real reaction conditions.

Key words: Operando DB-FTIR, Gas-phase molecular vibration spectroscopy, Heat irradiation influence, Real-time spectrum, Real reaction condition, Heterogeneous catalysis, Aromatization, Nano-sized HZSM-5 zeolite

Jiaxu Liu, Jilei Wang, Wei Zhou, Cuilan Miao, Guang Xiong, Qin Xin, Hongchen Guo. Construction of an operando dual-beam fourier transform infrared spectrometer and its application in the observation of isobutene reactions over nano-sized HZSM-5 zeolite[J]. Chinese Journal of Catalysis, 2017, 38(1): 13-19.

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Construction of an operando dual-beam fourier transform infrared spectrometer and its application in the observation of isobutene reactions over nano-sized HZSM-5 zeolite

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