Probing the catalytic behavior of ZnO nanowire supported Pd1 single-atom catalyst for selected reactions

doi:10.1016/S1872-2067(17)62899-7

Abstract

Abstract:

We have dispersed individual Pd atoms onto ZnO nanowires (NWs) as single-atom catalysts (SACs) and evaluated their catalytic performance for several selected catalytic reactions. The Pd₁/ZnO SAC is highly active, stable, and selective towards CO₂ for steam reforming of methanol to produce hy-drogen. This catalyst system is active for oxidation of CO and H₂ but performs poorly for preferential oxidation of CO in hydrogen-rich stream primarily due to the strong competitive oxidation of H₂ on ZnO supported Pd₁ atoms. At ambient pressure, reverse water-gas-shift reaction occurs on the Pd₁/ZnO SAC. This series of tests of catalytic reactions clearly demonstrate the importance of se-lecting the appropriate metal and support to develop SACs for catalytic transformation of molecules.

Key words: Single-atom catalyst, Palladium, Znic oxide nanowire, Steam reforming of methanol, Carbon monoxide oxidation, Hydrogenation

Jia Xu, Yian Song, Honglu Wu, Jingyue Liu. Probing the catalytic behavior of ZnO nanowire supported Pd₁ single-atom catalyst for selected reactions[J]. Chinese Journal of Catalysis, 2017, 38(9): 1549-1557.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(17)62899-7

https://www.cjcatal.com/EN/Y2017/V38/I9/1549

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Probing the catalytic behavior of ZnO nanowire supported Pd₁ single-atom catalyst for selected reactions

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