One-step synthesis of Pt@ZIF-8 catalyst for the selective hydrogenation of 1,4-butynediol to 1,4-butenediol

doi:10.1016/S1872-2067(16)62497-X

Abstract

Abstract:

A catalyst consisting of platinum nanoparticles on a ZIF-8 support(Pt@ZIF-8) was synthesized in a straightforward one-step procedure, by adding a nanostructured platinum sol during the formation of ZIF-8 at room temperature. Pt@ZIF-8 was highly porous and well crystallized. The Pt nanoparticles were well dispersed within the ZIF-8 support. In the hydrogenation of 1,4-butynediol, Pt@ZIF-8 exhibited high activity, excellent selectivity for 1,4-butenediol of greater than 94%, and reusability. The Pt@ZIF-8 catalyst did not require further additives. The favorable catalytic performance was attributed primarily to the modification of the ZIF-8 support by the platinum nanoparticles.

Key words: Platinum sol, ZIF-8, One-step synthesis, 1,4-Butynediol, Selective hydrogenation

Chuang Li, Mingming Zhang, Xin Di, Dongdong Yin, Wenzhen Li, Changhai Liang. One-step synthesis of Pt@ZIF-8 catalyst for the selective hydrogenation of 1,4-butynediol to 1,4-butenediol[J]. Chinese Journal of Catalysis, 2016, 37(9): 1555-1561.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(16)62497-X

https://www.cjcatal.com/EN/Y2016/V37/I9/1555

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