Chinese Journal of Catalysis ›› 2017, Vol. 38 ›› Issue (10): 1711-1718.DOI: 10.1016/S1872-2067(17)62907-3

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One-step synthesis of graphitic carbon nitride nanosheets for efficient catalysis of phenol removal under visible light

Wang Ding, Suqin Liu, Zhen He   

  1. College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, Hunan, China
  • Received:2017-04-21 Revised:2017-07-30 Online:2017-10-18 Published:2017-10-28
  • Contact: 10.1016/S1872-2067(17)62907-3

Abstract:

Graphitic carbon nitride (g-C3N4) nanosheet photocatalysts were synthesized via a facile impregnation-thermal method. The as-prepared materials were characterized and investigated as metal-free photocatalysts for the degradation of phenol in aqueous solution under visible light. Results revealed that the g-C3N4 nanosheets exhibited a 78.9% degradation for phenol after 30 min, which was much faster than that of the pristine g-C3N4. Using Brunauer-Emmett-Teller theory, the surface area of g-C3N4 nanosheets was 103.24 m2/g, which was much larger than that of g-C3N4. The larger surface area increases the contact area of the material with phenol, enhancing the photocatalytic activity. These results highlight the potential application of sustainable metal-free photocatalysts in water purification.

Key words: g-C3N4 nanosheet, Phenol degradation, Polymer, Semiconductor, Photocatalyst