Comparative study on the catalytic CO oxidation properties of CuO/CeO2 catalysts prepared by solid state and wet impregnation

doi:10.1016/S1872-2067(14)60138-8

Abstract

Abstract:

A series of CuO/CeO₂ catalysts were prepared by solid state impregnation (SSI) and wet impregnation (WI) methods and characterized by X-ray diffraction, H₂ temperature-programmed reduction (H₂-TPR), laser Raman spectroscopy (LRS), in situ diffuse reflectance infrared Fourier transform spectroscopy (in situ DRIFTS), and X-ray photoelectron spectroscopy (XPS). XPS and H₂-TPR results showed that SSI increased the dispersion of the copper species on the catalyst surface, which benefited the reduction of CuO species. LRS results indicated that a higher concentration of oxygen vacancies was obtained by the SSI method unlike the WI method. CO oxidation results showed that at a given CuO loading, the activity of the catalysts prepared by SSI was higher than that of their counterparts prepared by WI. Based on the combined characterization results, it was suggested that the enhanced activity was closely related to the higher concentrations of oxygen vacancies and Cu⁺-CO species on the catalysts. Last, a possible synergetic mechanism was proposed for CO oxidation over the CuO/CeO₂ catalysts.

Key words: Carbon monoxide oxidation, Copper oxide, Cerium oxide, Solid state impregnation, Wet impregnation, Synergistic mechanism

Jingfang Sun, Lei Zhang, Chengyan Ge, Changjin Tang, Lin Dong. Comparative study on the catalytic CO oxidation properties of CuO/CeO₂ catalysts prepared by solid state and wet impregnation[J]. Chinese Journal of Catalysis, 2014, 35(8): 1347-1358.

×
share this article

Add to citation manager EndNote|Ris|BibTeX

URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(14)60138-8

https://www.cjcatal.com/EN/Y2014/V35/I8/1347

References

[1] Feng Y F, Wang L, Zhang Y H, Guo Y, Guo Y L, Lu G Z, Chin J Catal (封雅芳, 王丽, 张艳慧, 郭耘, 郭扬龙, 卢冠忠. 催化学报), 2013, 34: 923
[2] Yuan Y Z, Kozlova A P, Asakura K, Wan H L, Tsai K, Iwasawa Y. J Catal, 1997, 170: 191
[3] Kuriyama M, Tanaka H, Ito S, Kubota T, Miyao T, Naito S, Tomi-shige K, Kunimori K. J Catal, 2007, 252: 39
[4] Zhu H Q, Qin Z F, Shan W J, Shen W J, Wang J G. Catal Today, 2007, 126: 382
[5] Tanaka H, Kuriyama M, Ishida Y, Ito S, Tomishige K, Kunimori K. Appl Catal A, 2008, 343: 117
[6] Zheng X C, Zhang X L, Wang S R, Yu L H, Wang X Y, Wu S H. Chin J Catal (郑修成, 张晓丽, 王淑荣, 于丽华, 王向宇, 吴世华. 催化学报), 2005, 26: 11
[7] Marinó F, Descorme C, Duprez D. Appl Catal B, 2005, 58: 175
[8] Liu W, Flytzani-Stephanopoulos M. J Catal 1995, 153: 317
[9] Avgouropoulos G, Ioannides T, Matralis H. Appl Catal B, 2005, 56: 87
[10] Gurbani A, Ayastuy J L, González-Marcos M P, Herrero J E, Guil J M, Gutiérrez-Ortiz M A. Int J Hydrogen Energy, 2009, 34: 547
[11] Jia A P, Hu G S, Meng L, Xie Y L, Lu J Q, Luo M F. J Catal, 2012, 289: 199
[12] Liu Z G, Zhou R X, Zheng X M. J Nat Gas Chem, 2008, 17: 125
[13] Gurbani A, Ayastuy J L, González-Marcos M P, Gutiérrez-Ortiz M A. Int J Hydrogen Energy, 2010, 35: 11582
[14] Zhou C F, Wang Y M, Cao Y, Zhuang T T, Huang W, Chun Y A, Zhu J H. J Mater Chem, 2006, 16: 1520
[15] Shon J K, Kong S S, Kim Y S, Lee J H, Park W K, Park S C, Kim J M. Microporous Mesoporous Mater, 2009, 120: 441
[16] Wang Y M, Wu Z Y, Wang H J, Zhu J H. Adv Funct Mater, 2006, 16: 2374
[17] Zheng M B, Cao J, Liao S T, Liu J S, Chen H Q, Zhao Y, Dai W J, Ji G B, Cao J M, Tao J. J Phys Chem C, 2009, 113: 3887
[18] Yue W, Zhou W Z. Chem Mater, 2007, 19: 2359
[19] Li X B, Quek X Y, Michel Ligthart D A J, Guo M L, Zhang Y, Li C, Yang Q H, Hensen E J M. Appl Catal B, 2012, 123: 424
[20] Medina-Mendoza A K, Cortés-Jácome M A, Toledo-Antonio J A, Angeles-Chávez C, López-Salinas E, Cuauhtémoc-López I, Barrera M C, Escobar J, Navarrete J, Hernández I. Appl Catal B, 2011, 106: 14
[21] Tang C J, Zhang H L, Sun C Z, Li J C, Qi L, Quan Y J, Gao F, Dong L. Catal Commun, 2011, 12: 1075
[22] Tang C J, Sun J F, Yao X J, Cao Y, Liu L C, Ge C Y, Gao F, Dong L. Appl Catal B, 2013, 146: 201
[23] Sun J F, Ge C Y, Yao X J, Cao Y, Zhang L, Tang C J, Dong L. Acta Phys-Chim Sin (孙敬方, 葛成艳, 姚小江, 曹原, 张雷, 汤常金, 董林. 物理化学学报), 2013, 29: 2451
[24] Mohamed M M, Salama T M, Othman A I, El-Shobaky G A. Appl Catal A, 2005, 279: 23
[25] Spanier J E, Robinson R D, Zhang F, Chan S W, Herman I P. Phys Rev B, 2001, 64: 245407
[26] Fernández-García M, Martínez-Arias A, Hanson J C, Rodriguez J A. Chem Rev, 2004, 104: 4063
[27] Qi L, Yu Q, Dai Y, Tang C J, Liu L J, Zhang H L, Gao F, Dong L, Chen Y. Appl Catal B, 2012, 119-120: 308
[28] Ilieva L, Pantaleo G, Ivanov I, Venezia A M, Andreeva D. Appl Catal B, 2006, 65: 101
[29] Liu L J, Yao Z J, Deng Y, Gao F, Liu B, Dong L. ChemCatChem, 2011, 3: 978
[30] Li X B, Quek X Y, Michel Ligthart D A J, Guo M L, Zhang Y, Li C, Yang Q H, Hensen E J M. Appl Catal B, 2012, 123-124: 424
[31] Liu Z G, Zhou R X, Zheng X M. Catal Commun, 2008, 9: 2183
[32] Tang X L, Zhang B C, Li Y, Xu Y D, Xin Q, Shen W J. Appl Catal A, 2005, 288: 116
[33] Park J W, Jeong J H, Yoon W L, Jung H, Lee H T, Lee D K, Park Y K, Rhee Y W. Appl Catal A, 2004, 274: 25
[34] Li L, Zhan Y Y, Zheng Q, Zheng Y H, Lin X Y, Li D L, Zhu J L. Catal Lett, 2007, 118: 91
[35] Moretti E, Storaro L, Talon A, Lenarda M, Riello P, Frattini R, del Valle Martínez de Yuso M, Jiménez-López A, Rodríguez-Castellón E, Ternero F, Caballero A, Holgado J P. Appl Catal B, 2011, 102: 627
[36] Yao X J, Gao F, Yu Q, Qi L, Tang C J, Dong L, Chen Y. Catal Sci Techol, 2013, 3: 1355
[37] Nelson A E, Schulz K H. Appl Surf Sci, 2003, 210: 206
[38] Gamarra D, Belver C, Fernández-García M, Martínez-Arías A. J Am Chem Soc, 2007, 129: 12064
[39] Gao X, Jiang Y, Zhong Y, Luo Z Y, Cen K F. J Hazard Mater, 2010, 174: 734
[40] Francisco M S P, Mastelaro V R, Nascente P A P, Florentino A O. J Phys Chem B, 2001, 105: 10515
[41] Cai W D, Chen F, Shen X X, Chen L J, Zhang J L. Appl Catal B, 2010, 101: 160
[42] Chang L H, Sasirekha N, Chen Y W, Wang W J. Ind Eng Chem Res, 2006, 45: 4927
[43] Gamarra D, Munuera G, Hungría A B, Fernández-García M, Conesa J C, Midgley P A. J Phys Chem C, 2007, 111: 11026
[44] Martínez-Arias A, Hungría A B, Fernández-García M, Conesa J C, Munuera G, Wang X Q, Harson J C, Rodriques J A, Martínez-Arias A. J Power Sources, 2005, 151: 32
[45] Bera P, López-Cámara A, Hornés A, Martínez-Arias A. J Phys Chem C, 2009, 113: 10689
[46] Meng M, Liu Y Q, Sun Z S, Zhang L J, Wang X T. Int J Hydrogen Energy, 2012, 37: 14133

Comparative study on the catalytic CO oxidation properties of CuO/CeO₂ catalysts prepared by solid state and wet impregnation

PDF (PC)

Knowledge

Abstract

Cite this article

share this article

share this article

References

Related Articles 15

Recommended Articles

Metrics

[1]	Haifeng Liu, Xiang Huang, Jiazang Chen. Surface electronic state modulation promotes photoinduced aggregation and oxidation of trace CO for lossless purification of H₂ stream [J]. Chinese Journal of Catalysis, 2023, 51(8): 49-54.
[2]	Ziye Zheng, Shuang Tian, Yuxiao Feng, Shan Zhao, Xin Li, Shuguang Wang, Zuoli He. Recent advances of photocatalytic coupling technologies for wastewater treatment [J]. Chinese Journal of Catalysis, 2023, 54(11): 88-136.
[3]	Linlin Wang, Xin Li, Leiduan Hao, Song Hong, Alex W. Robertson, Zhenyu Sun. Integration of ultrafine CuO nanoparticles with two-dimensional MOFs for enhanced electrochemical CO₂ reduction to ethylene [J]. Chinese Journal of Catalysis, 2022, 43(4): 1049-1057.
[4]	Yaroslava Lykhach, Tomá? Skála, Armin Neitzel, Nataliya Tsud, Klára Beranová, Kevin C. Prince, Vladimír Matolín, J?rg Libuda. Nanoscale architecture of ceria-based model catalysts: Pt-Co nanostructures on well-ordered CeO₂(111) thin films [J]. Chinese Journal of Catalysis, 2020, 41(6): 985-997.
[5]	Jiahua Zhao, Yuan Shu, Pengfei Zhang. Solid-state CTAB-assisted synthesis of mesoporous Fe₃O₄ and Au@Fe₃O₄ by mechanochemistry [J]. Chinese Journal of Catalysis, 2019, 40(7): 1078-1084.
[6]	Bing Han, Rui Lang, Hailian Tang, Jia Xu, Xiang-Kui Gu, Botao Qiao, Jingyue(Jimmy) Liu. Superior activity of Rh₁/ZnO single-atom catalyst for CO oxidation [J]. Chinese Journal of Catalysis, 2019, 40(12): 1847-1853.
[7]	Yuan Tan, Hua Liu, Xiao Yan Liu, Aiqin Wang, Changjun Liu, Tao Zhang. Effective removal of the protective ligands from Au nanoclusters by ambient pressure nonthermal plasma treatment for CO oxidation [J]. Chinese Journal of Catalysis, 2018, 39(5): 929-936.
[8]	Yan Gao, Hu Chen, Lu Ye, Zhongkai Lu, Yanan Yao, Yu Wei, Xuyang Chen. Highly effective electrochemical water oxidation by copper oxide film generated in situ from Cu(II) tricine complex [J]. Chinese Journal of Catalysis, 2018, 39(3): 479-486.
[9]	Lingxiang Wang, Liang Wang, Jian Zhang, Hai Wang, Feng-Shou Xiao. Enhancement of the activity and durability in CO oxidation over silica-supported Au nanoparticle catalyst via CeO_x modification [J]. Chinese Journal of Catalysis, 2018, 39(10): 1608-1614.
[10]	Jia Xu, Yian Song, Honglu Wu, Jingyue Liu. Probing the catalytic behavior of ZnO nanowire supported Pd₁ single-atom catalyst for selected reactions [J]. Chinese Journal of Catalysis, 2017, 38(9): 1549-1557.
[11]	Pengxin Liu, Jie Chen, Nanfeng Zheng. Photochemical route for preparing atomically dispersed Pd₁/TiO₂ catalysts on (001)-exposed anatase nanocrystals and P25 [J]. Chinese Journal of Catalysis, 2017, 38(9): 1574-1580.
[12]	SuHong Zhong, Guanzhong Lu, XueQing Gong. A DFT+U study of the structures and reactivities of polar CeO₂(100) surfaces [J]. Chinese Journal of Catalysis, 2017, 38(7): 1138-1147.
[13]	Shirish S. Punde, Bruce J. Tatarchuk. Pt-CeO₂/SiO₂ catalyst for CO oxidation in humid air at ambient temperature [J]. Chinese Journal of Catalysis, 2017, 38(3): 475-488.
[14]	Qi Yang, Linying Du, Xu Wang, Chunjiang Jia, Rui Si . CO oxidation over Au/ZrLa-doped CeO₂ catalysts: Synergistic effect of zirconium and lanthanum [J]. Chinese Journal of Catalysis, 2016, 37(8): 1331-1339.
[15]	Qi Sun, Xianglan Xu, Honggen Peng, Xiuzhong Fang, Wenming Liu, Jiawei Ying, Fan Yu, Xiang Wang . SnO₂-based solid solutions for CH₄ deep oxidation: Quantifying the lattice capacity of SnO₂ using an X-ray diffraction extrapolation method [J]. Chinese Journal of Catalysis, 2016, 37(8): 1293-1302.