Promotional effect of H3PO4 on ceria catalyst for selective catalytic reduction of NO by NH3

doi:10.1016/S1872-2067(15)60977-9

Abstract

Abstract:

A series of H₃PO₄-modified CeO₂ samples were prepared by impregnation of CeO₂ with H₃PO₄ solution, and evaluated for the selective catalytic reduction of NO_x by NH₃. The samples were characterized by X-ray diffraction, N₂ adsorption-desorption, infrared spectroscopy, Raman spectroscopy, X-ray photoelectron spectroscopy, temperature-programmed desorption of NH₃, and temperature-programmed reduction of H₂. The results showed that more than 80% NO conversion was achieved in the temperature range 250-550℃ over the H₃PO₄-CeO₂ catalyst. The enhanced catalytic performance could be ascribed to the increase in acidic strength, especially Brönsted acidity, and reduction in redox properties of the CeO₂ after H₃PO₄ modification.

Key words: Ammonia, Selective catalytic reduction, Ceria, Phosphoric acid, Redox, Acidity

Ting Yi, Yibo Zhang, Jingwei Li, Xiangguang Yang. Promotional effect of H₃PO₄ on ceria catalyst for selective catalytic reduction of NO by NH₃[J]. Chinese Journal of Catalysis, 2016, 37(2): 300-307.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(15)60977-9

https://www.cjcatal.com/EN/Y2016/V37/I2/300

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Promotional effect of H₃PO₄ on ceria catalyst for selective catalytic reduction of NO by NH₃

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