Versatile application of wet-oxidation for ambient CO abatement over Fe(OH)x supported subnanometer platinum group metal catalysts

doi:10.1016/S1872-2067(19)63489-3

Abstract

Abstract: The efficient and stable abatement of CO pollutant under ambient conditions is of great significance; however, it remains a formidable challenge. Herein, we report the versatile application of wet oxidation over Fe(OH)_x supported subnanometer Pt group metal (PGM) catalysts for the complete removal of CO under ambient temperature and humidity conditions. Typically, the 1.8 wt% Rh/Fe(OH)_x catalyst exhibited better durability during a~1400 min run for wet oxidation than for dry CO oxidation. Multiple characterization results including HR-TEM, H₂-TPR, and in-situ DRIFTS suggested that Fe(OH)_x, with good reducibility, promoted by the subnanometer Rh clusters, provided sites for the adsorption and reaction of O₂ and H₂O to form OH species. Subsequently, these OH species reacted with the adsorbed CO on Rh sites with a considerably lower activation energy (9 kJ mol^-1) than that of dissociated O species (22 kJ mol^-1), thus rationalizing the outstanding performance of Rh/Fe(OH)_x for wet oxidation. Extended experiments with other PGMs revealed a good generality for the application of wet oxidation in the efficient abatement of CO under humid conditions with Fe(OH)_x as the support.

Key words: Platinum group metals, CO, Oxidation, Ambient condition, Fe(OH)_x, Subnanometer clusters

Hongling Guan, Yang Chen, Chongyan Ruan, Jian Lin, Yang Su, Xiaodong Wang, Lingbo Qu. Versatile application of wet-oxidation for ambient CO abatement over Fe(OH)_x supported subnanometer platinum group metal catalysts[J]. Chinese Journal of Catalysis, 2020, 41(4): 613-621.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(19)63489-3

https://www.cjcatal.com/EN/Y2020/V41/I4/613

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Versatile application of wet-oxidation for ambient CO abatement over Fe(OH)_x supported subnanometer platinum group metal catalysts

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