Role of CeO2 in Three-Component Au/CeO2/SiO2 Composite Catalyst for Low-Temperature CO Oxidation

doi:10.1016/S1872-2067(11)60399-9

Abstract

Abstract: Hierarchical composite nanostructure composed of Au, CeO₂, and SiO₂ was fabricated by sequentially depositing ceria nanoparticles through impregnation and calcination, and then gold nanoparticles through a deposition-precipitation method on hierarchical monolithic silica (HMS) with multi-length scale pore structure. The Au/CeO₂/HMS composite nanostructure was characterized by X-ray diffraction, temperature-programmed reduction, and diffuse reflectance infrared Fourier transform spectroscopy. The results indicate that the presence of ceria had a significant effect on targeted deposition and stabilization of small metallic gold nanoparticles on the support. The temperature for complete conversion of CO to CO₂ over Au/CeO₂/HMS is ca. 60 ^oC at a space velocity of 80000 ml/(g·h). The highly dispersed metallic gold nanoparticles can activate CO and the small ceria nanoparticles supply oxygen in the reaction. The catalytic activity remains considerably stable during 48 h stability testing. The interaction between gold and ceria contributed greatly to CO oxidation and the presence of silica improved the stability of the gold catalyst.

Key words: silica, carbon monoxide oxidation, gold, ceria, stability

ZHANG Hui-Li, REN Li-Hui, LU An-Hui, LI Wen-Cui. Role of CeO₂ in Three-Component Au/CeO₂/SiO₂ Composite Catalyst for Low-Temperature CO Oxidation[J]. Chinese Journal of Catalysis, 2012, 33(7): 1125-1132.

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Role of CeO₂ in Three-Component Au/CeO₂/SiO₂ Composite Catalyst for Low-Temperature CO Oxidation

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